Abstract
We have demonstrated a highly efficient fully coherent 2D spectrometer based on 2D pulse shaping and Fourier beam shaping. The versatility of the design allows one to measure different 2D spectral surfaces consecutively. Easy alignment, inherent phase stability, rotating wave frame detection, and arbitrary waveform generation in all of the beams are important features of this design. We have demonstrated the functionality of the 2D spectrometer by measuring a 2D spectral surface of a GaAs quantum well.
Original language | English (US) |
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Pages (from-to) | 89-94 |
Number of pages | 6 |
Journal | Chemical Physics |
Volume | 341 |
Issue number | 1-3 |
DOIs | |
State | Published - Nov 15 2007 |
Keywords
- Coherent
- Four-wave mixing
- Multidimensional spectroscopy
- Pulse shaping
- Ultrafast spectroscopy
ASJC Scopus subject areas
- General Physics and Astronomy
- Physical and Theoretical Chemistry