Practical challenges in the development of photoelectrochemical solar fuels production

Mark T. Spitler, Miguel A. Modestino, Todd G. Deutsch, Chengxiang X. Xiang, James R. Durrant, Daniel V. Esposito, Sophia Haussener, Stephen Maldonado, Ian D. Sharp, Bruce A. Parkinson, David S. Ginley, Frances A. Houle, Thomas Hannappel, Nathan R. Neale, Daniel G. Nocera, Paul C. McIntyre

Research output: Contribution to journalReview articlepeer-review


This article addresses the challenges presented by photoelectrochemical solar fuels technology in a discussion that begins with a functioning device and proceeds to the more fundamental science of its component parts. In this flow of discussion issues are addressed that frame the discussion for the next, increasingly more fundamental topic. The analysis begins with a discussion of the need for an analytical facility for confirmation of reported efficiencies of solar fuels device prototypes and then progressively narrows its scope to prototype design, the discovery of novel materials and the design of durable interfacial structures for fuels evolution. Molecular hydrogen will be considered first as the target fuel since many of the challenges with hydrogen production are general and applicable to the more complex CO2 reduction, which will be treated as a supplementary subject.

Original languageEnglish (US)
Pages (from-to)985-995
Number of pages11
JournalSustainable Energy and Fuels
Issue number3
StatePublished - Mar 2020

ASJC Scopus subject areas

  • Renewable Energy, Sustainability and the Environment
  • Fuel Technology
  • Energy Engineering and Power Technology


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