Tandem catalysis and self-assembly: A one-pot approach to functionalized polymers

Joel M. Pollino; Marcus Weck

doi:10.1021/ol017205c

Tandem catalysis and self-assembly: A one-pot approach to functionalized polymers

Joel M. Pollino, Marcus Weck

Chemistry

Research output: Contribution to journal › Article › peer-review

Abstract

(equation presented) Side-chain functionalized polymers possessing terminal palladated SCS pincer complexes at each repeat unit were synthesized via ring-opening metathesis polymerization. These palladium centers function as both well-defined Heck catalysts and recognition units capable of quantitative self-assembly of pyridine-containing molecules. Exploitation of both the catalytic and self-assembly properties has led to the development of a controlled, one-pot tandem catalysis/self-assembly sequence for the synthesis of functionalized polymers.

Original language	English (US)
Pages (from-to)	753-756
Number of pages	4
Journal	Organic Letters
Volume	4
Issue number	5
DOIs	https://doi.org/10.1021/ol017205c
State	Published - Mar 7 2002

ASJC Scopus subject areas

Biochemistry
Physical and Theoretical Chemistry
Organic Chemistry

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10.1021/ol017205c

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title = "Tandem catalysis and self-assembly: A one-pot approach to functionalized polymers",

abstract = "(equation presented) Side-chain functionalized polymers possessing terminal palladated SCS pincer complexes at each repeat unit were synthesized via ring-opening metathesis polymerization. These palladium centers function as both well-defined Heck catalysts and recognition units capable of quantitative self-assembly of pyridine-containing molecules. Exploitation of both the catalytic and self-assembly properties has led to the development of a controlled, one-pot tandem catalysis/self-assembly sequence for the synthesis of functionalized polymers.",

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AU - Weck, Marcus

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N2 - (equation presented) Side-chain functionalized polymers possessing terminal palladated SCS pincer complexes at each repeat unit were synthesized via ring-opening metathesis polymerization. These palladium centers function as both well-defined Heck catalysts and recognition units capable of quantitative self-assembly of pyridine-containing molecules. Exploitation of both the catalytic and self-assembly properties has led to the development of a controlled, one-pot tandem catalysis/self-assembly sequence for the synthesis of functionalized polymers.

AB - (equation presented) Side-chain functionalized polymers possessing terminal palladated SCS pincer complexes at each repeat unit were synthesized via ring-opening metathesis polymerization. These palladium centers function as both well-defined Heck catalysts and recognition units capable of quantitative self-assembly of pyridine-containing molecules. Exploitation of both the catalytic and self-assembly properties has led to the development of a controlled, one-pot tandem catalysis/self-assembly sequence for the synthesis of functionalized polymers.

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JO - Organic Letters

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Tandem catalysis and self-assembly: A one-pot approach to functionalized polymers

Abstract

ASJC Scopus subject areas

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